Research
The majority of plastic waste is landfilled, burned or leaks to the environment. Unfortunately, only 12 % (by weight) is recycled globally1 mainly because the predominantly applied recycling technique of melting and re-extrusion produces a lower quality plastic.2–6 Therefore, chemical depolymerization of plastic has been studied to produce monomers which can be used to make high-quality plastic again. For polyolefins, however, only a very mixed, low value hydrocarbon stream was obtained thus far.4 This is because thermal cracking of the strong polyolefin bonds evokes random bond scission, uncontrolled further reaction and thus the formation of various products besides monomers.
My research focusses on developing pathways for the low temperature selective chemical recycling of plastic waste to chemical building blocks like aromatics, carboxylic acids and monomers. I am especially interested in using mechanochemistry and catalysis to drive the depolymerization and cracking reactions of polyolefins. Mechanochemistry is a rather less developed field of chemistry where reactions are driven not by thermal energy, electrons or photons but rather by mechanical strain, which can lower the activation energy needed to be overcome for bond cleavage. This strain can, for example, be applied in a ball mill. Heterogeneous catalysts can also lower the activation energy barrier and improve selectivity to commercially interesting products like aromatics.
Extending the bonds of polymers by force, e.g. in a ball mill can assist their cleavage and help to depolymerize them at lower temperatures.
(1) The Ellen MacArthur Foundation. The New Plastics Economy: Rethinking the Future of Plastic&Catalysing Action; 2013; Vol. 52.
(2) Jansson, A.; Möller, K.; Gevert, T. Degradation of Post-Consumer Polypropylene Materials Exposed to Simulated Recycling—Mechanical Properties. Polym. Degrad. Stab. 2003, 82 (1), 37–46. https://doi.org/10.1016/S0141-3910(03)00160-5.
(3) Canevarolo, S. V. Chain Scission Distribution Function for Polypropylene Degradation during Multiple Extrusions. Polym. Degrad. Stab. 2000, 70(1), 71–76. https://doi.org/10.1016/S0141-3910(00)00090-2.
(4) Ragaert, K.; Delva, L.; Van Geem, K. Mechanical and Chemical Recycling of Solid Plastic Waste. Waste Manag. 2017, 69, 24–58. https://doi.org/10.1016/j.wasman.2017.07.044.
(5) Dordinejad, A. K.; Sharif, F.; Ebrahimi, M.; Rashedi, R. Rheological and Thermorheological Assessment of Polyethylene in Multiple Extrusion Process. Thermochim. Acta 2018, 668, 19–27. https://doi.org/10.1016/J.TCA.2018.08.010.
(6) Bai, C.; Spontak, R. J.; Koch, C. C.; Saw, C. K.; Balik, C. M. Structural Changes in Poly(Ethylene Terephthalate) Induced by Mechanical Milling. Polymer (Guildf). 2000, 41 (19), 7147–7157. https://doi.org/10.1016/S0032-3861(00)00048-3.
C.V.
2015 – 2019 PhD at Technical University Delft in Catalysis Engineering
2013 -2015 M.S.CEP Chemical Engineering at Massachusetts Institute of Technology
2009 – 2013 B.Sc. Process Engineering University of Applied Sciences Hamburg
Aydonat, Simay; Hergesell, Adrian H.; Seitzinger, Claire L.; Lennarz, Regina; Chang, George; Sievers, Carsten; Meisner, Jan; Vollmer, Ina; Göstl, Robert
Leveraging mechanochemistry for sustainable polymer degradation Journal Article
In: Polymer Journal, 2024, (Cited by: 0; All Open Access, Hybrid Gold Open Access).
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Vollmer, Ina; Jenks, Michael J. F.; Rejman, Sebastian; Meirer, Florian; Gurinov, Andrei; Baldus, Marc; Weckhuysen, Bert M.
Unravelling potential reaction intermediates during catalytic pyrolysis of polypropylene with microscopy and spectroscopy Journal Article
In: Catalysis Science and Technology, vol. 52, 2024, (Cited by: 0; All Open Access, Hybrid Gold Open Access).
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Schnabl, Kordula B.; Mandemaker, Laurens D. B.; Nierop, Klaas G. J.; Deen, Olivier V. B.; Eefting, Desmond D.; Vollmer, Ina; Weckhuysen, Bert M.
Green Additives in Chitosan-Based Bioplastic Films: Physical, Mechanical, and Chemical Properties Journal Article
In: ChemSusChem, vol. 16, no. 20, 2023, (Cited by: 0; All Open Access, Hybrid Gold Open Access).
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title = {Green Additives in Chitosan-Based Bioplastic Films: Physical, Mechanical, and Chemical Properties},
author = { Kordula B. Schnabl and Laurens D. B. Mandemaker and Klaas G. J. Nierop and Olivier V. B. Deen and Desmond D. Eefting and Ina Vollmer and Bert M. Weckhuysen},
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Vollmer, Ina; Sardon, Haritz; Huber, George W.; Li, Zhibo
Introduction to Plastic Conversion Journal Article
In: Polymer Chemistry, vol. 14, no. 26, pp. 3054 – 3056, 2023, (Cited by: 0).
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Thevenon, Arnaud; Vollmer, Ina
Towards a Cradle-to-Cradle Polyolefin Lifecycle Journal Article
In: Angewandte Chemie - International Edition, vol. 62, no. 3, 2023, (Cited by: 2).
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Vollmer, Ina; Sardon, Haritz; Huber, George W.; Li, Zhibo
Introduction to Plastic Conversion Journal Article
In: Catalysis Science and Technology, vol. 13, no. 13, pp. 3737 – 3739, 2023, (Cited by: 0).
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Jöbsis, Huygen J.; Fykouras, Kostas; Reinders, Joost W. C.; van Katwijk, Jacco; Dorresteijn, Joren M.; Arens, Tjom; Vollmer, Ina; Muscarella, Loreta A.; Leppert, Linn; Hutter, Eline M.
Conduction Band Tuning by Controlled Alloying of Fe into Cs2AgBiBr6 Double Perovskite Powders Journal Article
In: Advanced Functional Materials, 2023, (Cited by: 1; All Open Access, Green Open Access, Hybrid Gold Open Access).
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Smak, Tom J.; de Peinder, Peter; der Waal, Jan C. Van; Altink, Rinke; Vollmer, Ina; Weckhuysen, Bert M.
Oxidative Conversion of Polyethylene Towards Di-Carboxylic Acids: A Multi-Analytical Approach Journal Article
In: ChemSusChem, 2023, (Cited by: 0).
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Rejman, Sebastian; Vollmer, Ina; Werny, Maximilian J.; Vogt, Eelco T. C.; Meirer, Florian; Weckhuysen, Bert M.
Transport limitations in polyolefin cracking at the single catalyst particle level Journal Article
In: Chemical Science, vol. 14, no. 37, pp. 10068 – 10080, 2023, (Cited by: 4; All Open Access, Gold Open Access, Green Open Access).
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title = {Transport limitations in polyolefin cracking at the single catalyst particle level},
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Vaksmaa, Annika; Knittel, Katrin; Asbun, Alejandro Abdala; Goudriaan, Maaike; Ellrott, Andreas; Witte, Harry J.; Vollmer, Ina; Meirer, Florian; Lott, Christian; Weber, Miriam; Engelmann, Julia C.; Niemann, Helge
Microbial Communities on Plastic Polymers in the Mediterranean Sea Journal Article
In: Frontiers in Microbiology, vol. 12, 2021, (Cited by: 54; All Open Access, Gold Open Access, Green Open Access).
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title = {Microbial Communities on Plastic Polymers in the Mediterranean Sea},
author = { Annika Vaksmaa and Katrin Knittel and Alejandro Abdala Asbun and Maaike Goudriaan and Andreas Ellrott and Harry J. Witte and Ina Vollmer and Florian Meirer and Christian Lott and Miriam Weber and Julia C. Engelmann and Helge Niemann},
url = {https://www.scopus.com/inward/record.uri?eid=2-s2.0-85109015565&doi=10.3389%2ffmicb.2021.673553&partnerID=40&md5=6ca30a15f9c1b31221ad5b30aca36c15},
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Vollmer, Ina; Jenks, Michael J. F.; González, Rafael Mayorga; Meirer, Florian; Weckhuysen, Bert M.
Plastic Waste Conversion over a Refinery Waste Catalyst Journal Article
In: Angewandte Chemie - International Edition, vol. 60, no. 29, pp. 16101 – 16108, 2021, (Cited by: 68; All Open Access, Green Open Access, Hybrid Gold Open Access).
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Vollmer, Ina; Jenks, Michael J. F.; Roelands, Mark C. P.; White, Robin J.; van Harmelen, Toon; de Wild, Paul; van der Laan, Gerard P.; Meirer, Florian; Keurentjes, Jos T. F.; Weckhuysen, Bert M.
Beyond Mechanical Recycling: Giving New Life to Plastic Waste Journal Article
In: Angewandte Chemie - International Edition, vol. 59, no. 36, pp. 15402 – 15423, 2020, (Cited by: 695; All Open Access, Green Open Access).
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url = {https://www.scopus.com/inward/record.uri?eid=2-s2.0-85087630608&doi=10.1002%2fanie.201915651&partnerID=40&md5=c90b03bdfab6b6c73c6e8241b29e7914},
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Yarulina, I; Wispelaere, K De; Bailleul, S; Goetze, J; Radersma, M; Abou-Hamad, E; Vollmer, I; Goesten, M; Mezari, B; Hensen, E J M; Martínez-Espín, J S; Morten, M; Mitchell, S; Perez-Ramirez, J; Olsbye, U; Weckhuysen, B M; Speybroeck, V Van; Kapteijn, F; Gascon, J
Erratum to: Structure–performance descriptors and the role of Lewis acidity in the methanol-to-propylene process (Nature Chemistry, (2018), 10, 8, (804-812), 10.1038/s41557-018-0081-0) Journal Article
In: Nature Chemistry, vol. 10, no. 8, pp. 897, 2018, (cited By 1).
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Yarulina, I; Wispelaere, K De; Bailleul, S; Goetze, J; Radersma, M; Abou-Hamad, E; Vollmer, I; Goesten, M; Mezari, B; Hensen, E J M; Martínez-Espín, J S; Morten, M; Mitchell, S; Perez-Ramirez, J; Olsbye, U; Weckhuysen, B M; Speybroeck, V Van; Kapteijn, F; Gascon, J
Structure–performance descriptors and the role of Lewis acidity in the methanol-to-propylene process Journal Article
In: Nature Chemistry, vol. 10, no. 8, pp. 804-812, 2018, (cited By 84).
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Yarulina, Irina; Wispelaere, Kristof De; Bailleul, Simon; Goetze, Joris; Radersma, Mike; Abou-Hamad, Edy; Vollmer, Ina; Goesten, Maarten; Mezari, Brahim; Hensen, Emiel J. M.; Martínez-Espín, Juan S.; Morten, Magnus; Mitchell, Sharon; Perez-Ramirez, Javier; Olsbye, Unni; Weckhuysen, Bert M.; Speybroeck, Veronique Van; Kapteijn, Freek; Gascon, Jorge
Erratum to: Structure–performance descriptors and the role of Lewis acidity in the methanol-to-propylene process (Nature Chemistry, (2018), 10, 8, (804-812), 10.1038/s41557-018-0081-0) Journal Article
In: Nature Chemistry, vol. 10, no. 8, pp. 897, 2018, (Cited by: 4; All Open Access, Bronze Open Access).
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title = {Erratum to: Structure–performance descriptors and the role of Lewis acidity in the methanol-to-propylene process (Nature Chemistry, (2018), 10, 8, (804-812), 10.1038/s41557-018-0081-0)},
author = { Irina Yarulina and Kristof De Wispelaere and Simon Bailleul and Joris Goetze and Mike Radersma and Edy Abou-Hamad and Ina Vollmer and Maarten Goesten and Brahim Mezari and Emiel J. M. Hensen and Juan S. Martínez-Espín and Magnus Morten and Sharon Mitchell and Javier Perez-Ramirez and Unni Olsbye and Bert M. Weckhuysen and Veronique Van Speybroeck and Freek Kapteijn and Jorge Gascon},
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Vollmer, Ina; Li, Guanna; Yarulina, Irina; Kosinov, Nikolay; Hensen, Emiel J.; Houben, Klaartje; Mance, Deni; Baldus, Marc; Gascon, Jorge; Kapteijn, Freek
Relevance of the Mo-precursor state in H-ZSM-5 for methane dehydroaromatization Journal Article
In: Catalysis Science and Technology, vol. 8, no. 3, pp. 916 – 922, 2018, (Cited by: 42; All Open Access, Green Open Access).
@article{Vollmer2018916,
title = {Relevance of the Mo-precursor state in H-ZSM-5 for methane dehydroaromatization},
author = { Ina Vollmer and Guanna Li and Irina Yarulina and Nikolay Kosinov and Emiel J. Hensen and Klaartje Houben and Deni Mance and Marc Baldus and Jorge Gascon and Freek Kapteijn},
url = {https://www.scopus.com/inward/record.uri?eid=2-s2.0-85041510829&doi=10.1039%2fc7cy01789h&partnerID=40&md5=e402a23869c72631afa91abb7232ae0a},
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Yarulina, Irina; Wispelaere, Kristof De; Bailleul, Simon; Goetze, Joris; Radersma, Mike; Abou-Hamad, Edy; Vollmer, Ina; Goesten, Maarten; Mezari, Brahim; Hensen, Emiel J. M.; Martínez-Espín, Juan S.; Morten, Magnus; Mitchell, Sharon; Perez-Ramirez, Javier; Olsbye, Unni; Weckhuysen, Bert M.; Speybroeck, Veronique Van; Kapteijn, Freek; Gascon, Jorge
Structure–performance descriptors and the role of Lewis acidity in the methanol-to-propylene process Journal Article
In: Nature Chemistry, vol. 10, no. 8, pp. 804 – 812, 2018, (Cited by: 209; All Open Access, Green Open Access).
@article{Yarulina2018804,
title = {Structure–performance descriptors and the role of Lewis acidity in the methanol-to-propylene process},
author = { Irina Yarulina and Kristof De Wispelaere and Simon Bailleul and Joris Goetze and Mike Radersma and Edy Abou-Hamad and Ina Vollmer and Maarten Goesten and Brahim Mezari and Emiel J. M. Hensen and Juan S. Martínez-Espín and Magnus Morten and Sharon Mitchell and Javier Perez-Ramirez and Unni Olsbye and Bert M. Weckhuysen and Veronique Van Speybroeck and Freek Kapteijn and Jorge Gascon},
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Other publications
See earlier publications on Scopus.
